- (1993) Recorded "William Shatner and Leonard Nimoy Read Four Science Fiction Classics" featuring stories by Isaac Asimov, Ray Bradbury, Henry Kuttner and Robert A. Heinlein.
- (1974) Poetry book: "Warmed By Love".
- (2000s) Audiobook: Narrates "Alien Voices Presents H.G. Wells' 'The Time Machine'".
- (1997) Audiobook: Narrated "Star Trek: Vulcan's Forge".
- Created the "Primortals" comic book series.
- TV commercial: Oldsmobile cars ("This is not your father's Oldsmobile" with daughter Julie Nimoy).
- Narrated the "New England Time Capsule" Omnimax film for the Boston Museum of Science.
- (Late 1960s-early 1970s) Recorded several albums of folk-rock including camp classic versions of "Proud Mary" and "The Ballad of Bilbo Baggins" (some of these songs were issued in the 1990s on the CD "Spaced Out").
- Video game: Narrated the English-language version of the Sega Dreamcast video game "Seaman."
- (1983) Hosted a one-hour retrospective on Star Trek (1966). This special has since been added to some syndication packages of "Star Trek".
- (1984) Music video: Directed / appeared in The Bangles video "Going Down to Liverpool".
- (1987) Album: Narrated "Whales Alive" by Paul Winter and Paul Halley. NOTE: The album was made to call attention to the endangerment of whales and was released to capitalize on the themes of Star Trek IV: The Voyage Home (1986)).
- (1960s) Music video: In circulation showing him lip-synching "Ballad of Bilbo Baggins" on a 1960s TV show.
- (2004) TV commercial: Priceline.com (with William Shatner).
- Record: Played "Mr. Spock" on a live recording with John de Lancie, "Spock vs. Q".
- Audio CD: "William Shatner and Leonard Nimoy Read 4 Science Fiction Classics: Foundation, Psychohistorians, Mimsy Were The Borogoves, and Martian Chronicles."
- (10/89) Audio CD: Narrates, with J.M. Dillard and James Doohan, "Star Trek: The Lost Years".
- (2004) TV commercial: Aleve pain relief medication.
- (1970s) Magazine advertisement: Celestron telescopes.
- (10/06) TV commercial: DirecTV as Capt. Spock from Star Trek VI: The Undiscovered Country (1991); appears on the bridge of the Starship Enterprise with William Shatner as Capt. James T. Kirk, DeForest Kelley as Dr. Leonard "Bones" McCoy, James Doohan as Capt. Montgomery "Scotty" Scott, Walter Koenig as Cmdr. Pavel Chekov, Nichelle Nichols as Cmdr. Uhura, George Takei as Capt. Hikaru Sulu and Kim Cattrall as Lt. Valeris.
- (10/89) Audio book: Narrates, with J.M. Dillard, "Star Trek V".
- (1988) TV commercial (PSA): various childhood diseases.
- (2003) Referenced by 'Weird Al' Yankovic on the track "Albquerque" on his CD "Poodle Hat".
- (2006) TV commercials (PSAs): Amnesty International.
- Video game: Narrates "Sid Meier's Civilization IV".
- (Late 1980s) Audiobook: Provided the voice of Spock in audio adaptation of "Star Trek" novel "Star Trek IV: The Voyage Home".
- (Late 1980s) Audiobook: Provided the voice of Spock in audio adaptation of "Star Trek" novel "Strangers from the Sky".
- (Late 1980s) Audiobook: Provided the voice of Spock in audio adaptation of "Star Trek" novel "Yesterday's Son".
- (Late 1980s) Audiobook: Provided the voice of Spock in audio adaptation of "Star Trek" novel "The Entropy Effect".
- (2000s) Audiobook: Narrates "Alien Voices Presents Sir Arthur Conan Doyle's 'The Lost World'".
- (2000s) Audiobook: Narrates "Alien Voices Presents H.G. Wells' 'War of the Worlds'".
- (2000s) Audiobook: Narrates "Alien Voices Presents Jules Verne 'Journey to the Center of the Earth'".
- (1998) Foreword: Wrote the foreword for Grace Lee Whitney's autobiography, "The Longest Trek: My Tour of the Galaxy".
- Poetry book: "You and I".
- (1974) Poetry book: "Will I Think of You?".
- (1977) Book: "We Are All Searching for Love: A Collection of Poems and Photographs".
- Poetry book: "These Words Are For You".
- (1978) Poetry book: "Come Be With Me".
- (1988) Music video: His voice from Errand of Mercy (1967) speaking the phrase, "Pure energy" was used in the Information Society video "What's on Your Mind (Pure Energy)".
- Stage: Appeared in "Equus" on Broadway.
- Stage: Appeared in "Camelot" on Broadway.
- Stage: Appeared in "Oliver" on Broadway.
- Stage: Appeared in "Fiddler on the Roof" on Broadway.
- (3/22/79) Guest on the daytime program "Afternoon Exchange" talking about the play "Vincent" which he starred in at the Drury Playhouse.
- (5/29/89) Guest on "Live on Five" talking about Star Trek V: The Final Frontier (1989).
- (2014) TV commercial: Volkswagen Golf automobile.
- Record: Played "Mr. Spock" on a live recording with John de Lancie, entitled "Spock vs. Q: The Sequel".
- (1966) Unsold pilot: Appeared in a pilot for a proposed adventure series to be called "Stranded".
- (11/26-75-12/21/785) Stage: Appeared (as "Malvolio") in William Shakespeare's play, "Twelfth Night," at the Public Theater in Pittsburgh, PA. Ben Shaktman was director.
- (1967) Single: Hit #121 on the Billboard Singles Chart with "Visit to a Sad Planet" (Dot 17038).
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