- Buckley graduated from The Royal Academy of Dramatic Art in January 2013.
- In the 2013 summer season at Shakespeare's Globe she played Miranda in The Tempest, and singer Arabella Hunt and Kate in Samuel Adamson's Gabriel.
- After coming second in the 'I'd Do Anything' search for Nancy, she was offered the alternate role of Nancy (having been Andrew Lloyd Webber and Cameron Mackintosh's favorite to win the competition), but she turned it down, deciding instead to appear in an Off-West End production of 'A Little Night Music', which eventually transferred to the Garrick Theatre (and subsequently to Broadway, with a different cast).
- Invited to join the actor's branch of AMPAS in 2022.
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